24-28 Sep 2017 Saint Malo (France)

Author index > Takubo Yusaku

Sound velocity and elastic properties of liquid Fe–Ni–Si at high pressure
Hidenori Terasaki  1@  , Mayumi Maki  2@  , Yuta Shimoyama  2@  , Keisuke Nishida  3@  , Satoru Urakawa  4@  , Yusaku Takubo  2@  , Yuki Shibazaki  5@  , Tatsuya Sakamaki  6@  , Yuji Higo  7@  , Akihiko Machida  8@  , Tadashi Kondo  2@  
1 : Department of Earth and Space Science, Graduate School of Science, Osaka University  (Osaka Univ.)
2 : Department of Earth and Space Science, Graduate School of Science, Osaka University
3 : Department of Earth and Planetary Science, Graduate School of Science, The University of Tokyo  (The univ. of Tokyo)
7-3-1 Hongo Bunkyo-ku 113-0033 Tokyo -  Japan
4 : Department of Earth Science, Okayama University
5 : Frontier Research Institute for Interdisciplinary Sciences, Tohoku University  (Tohoku Univ.)
6 : Department of Earth Sciences, Tohoku University
7 : Japan Synchrotron Radiation Institute  (JASRI)
8 : National Institutes for Quantum and Radiological Science and Technology

Sound velocity, density, and elastic properties, such as bulk modulus, of liquid Fe-alloys at high pressure give us important information to constrain interior structures and composition of molten cores of terrestrial planets. Si is one of the major light elements in the planetary core. Here, we measured compressional wave velocity (Vp) and density of liquid Fe–Ni–Si and studied the effect of pressure, temperature, and Si content on these properties.

Sound velocity and density of liquid Fe52Ni10Si38 was measured up to 12 GPa and 2100 K using ultrasonic pulse-echo method and X-ray absorption method, respectively. The measurements were carried out at BL04B1 and BL22XU beamlines, SPring-8.

The measured Vp of Fe–Ni–Si is larger than that of liquid Fe (Jing et al. 2014) and Fe–Ni (Kuwabara et al. 2016) in all the pressure range studied. The effect of Si on the Vp is opposite to that of S at present pressure conditions. The Vp of liquid Fe–Ni–Si decreases slightly with increasing temperature and the dVp/dT of this study is in agreement with that measured at ambient pressure (Williams et al. 2015). The adiabatic bulk modulus (Ks0) at ambient pressure and its pressure derivative (Ks') were obtained by fitting the Vp data using the Birch-Murnaghan and Vinet equation of state. The obtained Ks0 of liquid Fe–Ni–Si is close to that of liquid Fe–Ni (Kuwabara et al. 2016). The calculated density from the Ks0 and Ks' shows a good agreement with the directly measured density.

 

Refs.

Jing et al. (2014) Earth Planet. Sci. Lett. 396, 78-87.

Kuwabara et al. (2016) Phys. Chem. Mineral. 89, 273-276.

Williams et al. (2015) J. Geophys. Res. Solid Earth, 120, 6846–6855.


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